Ah, excellent question, Lalaith! That is indeed an important question for translators not only of books, but also of movie dialogues for dubbing. Just where does the relationship turn personal enough to allow a transition from the formal "Sie" to the intimate "du"? Basically, one can only attempt to locate a point of time in the plot where the change would take place if it were originally written in German. That also depends on the historical period in which the story takes place. The use of the second person personal pronoun has changed in history.
The medieval feeling of LotR means that there is a form that was once used and is now considered old-fashioned, if not obsolete - "Ihr". That is what Sam uses for "Herr Gandalf". I don't have the modern German translation, so I don't know off-hand what he uses there. But a modern usage would change the flavour of the story, taking it out of ancient times.
Tolkien did give us a hint about the Hobbits' usage - he once said/wrote (sorry, I don't have the exact quote or location at the moment) that the Hobbits only use the familiar pronoun. For that reason Pippin was considered royalty by the people of Gondor, because he addressed Denethor with the familiar pronoun! Only an equal would be allowed that privilege.
That is the reason that Sam calls Frodo "Herr Frodo" (Mr. Frodo) yet uses the familiar "du" - an unlikely combination!
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'Mercy!' cried Gandalf. 'If the giving of information is to be the cure of your inquisitiveness, I shall spend all the rest of my days in answering you. What more do you want to know?' 'The whole history of Middle-earth.. .'
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